www.geologicacarpathica.sk
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, AUGUST 2012, 63, 4, 335—342 doi: 10.2478/v10096-012-0026-2
Burial history, thermal history and hydrocarbon generation
modelling of the Jurassic source rocks in the basement of the
Polish Carpathian Foredeep and Outer Carpathians
(SE Poland)
PAWEŁ KOSAKOWSKI and MAGDALENA WRÓBEL
AGH University of Science and Technology, Faculty of Geology, Geophysics and Environmental Protection, Al. Mickiewicza 30,
30-059 Kraków, Poland; kosak@agh.edu.pl; wrobelm@agh.edu.pl
(Manuscript received November 22, 2011; accepted in revised form March 13, 2012)
Abstract: Burial history, thermal maturity, and timing of hydrocarbon generation were modelled for the Jurassic source
rocks in the basement of the Carpathian Foredeep and marginal part of the Outer Carpathians. The area of investigation
was bounded to the west by Kraków, to the east by Rzeszów. The modelling was carried out in profiles of wells:
Będzienica 2, Dębica 10K, Góra Ropczycka 1K, Goleszów 5, Nawsie 1, Pławowice E1 and Pilzno 40. The organic matter,
containing gas-prone Type III kerogen with an admixture of Type II kerogen, is immature or at most, early mature to
0.7 % in the vitrinite reflectance scale. The highest thermal maturity is recorded in the south-eastern part of the study
area, where the Jurassic strata are buried deeper. The thermal modelling showed that the obtained organic matter matu-
rity in the initial phase of the “oil window” is connected with the stage of the Carpathian overthrusting. The numerical
modelling indicated that the onset of hydrocarbon generation from the Middle Jurassic source rocks was also connected
with the Carpathian thrust belt. The peak of hydrocarbon generation took place in the orogenic stage of the overthrusting.
The amount of generated hydrocarbons is generally small, which is a consequence of the low maturity and low transfor-
mation degree of kerogen. The generated hydrocarbons were not expelled from their source rock. An analysis of matu-
rity distribution and transformation degree of the Jurassic organic matter shows that the best conditions for hydrocarbon
generation occurred most probably in areas deeply buried under the Outer Carpathians. It is most probable that the
“generation kitchen” should be searched for there.
Key words: Jurassic, Outer Carpathians, Carpathian Foredeep, SE Poland, 1-D modelling, source rocks, generation.
Introduction
The study area located between Kraków and Rzeszów (Fig. 1)
has been subjected to intensive drilling exploration since the
1950s. As a result, many natural gas deposits have been dis-
covered within the Miocene cover (Kotarba & Peryt 2011).
The gases accumulated there are microbial, that is formed be-
fore the thermogenic processes (Kotarba 2011). Numerous
small commercial and uncommercial oil and gas accumula-
tions have also been discovered within the Upper Jurassic—
Lower Cretaceous carbonate complex and Upper Cretaceous
carbonate and clastic complexes (Karnkowski 1993; Myśliwiec
et al. 2006). The Upper Jurassic (—Lower Cretaceous) carbon-
ates were found to contain an oil accumulation in the Partynia-
Podborze field, gas accumulations in the Wojsław, Łączki
Brzeskie, and Mędrzechów fields, oil and gas accumulation in
the Korzeniów-Męciszów, and gas-condensate accumulations
in the Góra Ropczycka and Tarnów fields (Myśliwiec et al.
2006; Kotarba et al. 2011). In both the Upper Jurassic and
Upper Cretaceous strata the hydrocarbon accumulations were
found in the Dąbrowa Tarnowska and Grobla-Pławowice
fields (oils and gas), Łapanów (gas), Łąkta (gas and conden-
sate), Smęgorzów (gas), and Żukowice fields (gas). The Upper
Cretaceous sandstones were found to contain gas accumula-
tions in the Brzezowiec, Jastrząbka Stara, Rajsko, Rylowa, and
Swarzów fields (Karnkowski 1993; Myśliwiec et al. 2006).
Gases occurring in the Paleozoic-Mesozoic basement of the
Polish Carpathian Foredeep are both microbial and thermo-
genic (Kotarba 2012).
Due to a significant incompleteness of the sedimentation
profile, caused mainly by erosional processes, it is important
to define the source of the hydrocarbon mass accumulated
later in reservoir rocks and to reconstruct the course of the
processes.
In the current work, the generation potential of the Jurassic
strata of the basement of the Carpathian Foredeep and the
marginal part of the Outer Carpathians was evaluated in the
area between Kraków and Rzeszów, with the use of 1-D
modelling methods. The analysis was carried out in the
Będzienica 2, Dębica 10K, Góra Ropczycka 1K, Goleszów 5,
Nawsie 1, Pławowice E1 and Pilzno 40 wells (Fig. 1).
Outline of geology
The study area comprises the Mesozoic cover within the
range of the basement of the Carpathian Foredeep and the
marginal part of the Outer Carpathians between Kraków and
Rzeszów (Fig. 1). Its western boundary reaches the Kraków-
Lubliniec Fold Zone and corresponds to the boundary of the
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Paleozoic structural unit called the Małopolska Block. Its
eastern boundary is the Lower San Horst Structure (Fig. 1).
The basement of the Carpathian Foredeep and the Outer
Carpathians is composed of the Lower Paleozoic strata form-
ing the Caledonian structural stage, the Upper Paleozoic
strata forming the Variscan stage, and the Permian and
Mesozoic strata forming the Alpine structural stage. A de-
scription of the Caledonian and Variscan stages in the study
area can be found in Buła & Habryn (2008, 2011) and
Kosakowski & Wróbel (2011), and the Alpine stage adopted for
the purposes of the modelling of hydrocarbon generation and
expulsion processes is given as in Oszczypko et al. (2006),
Świdrowska et al. (2008) and Kosakowski et al. (2011).
The Mesozoic strata form three complexes: the Permian—
Triassic, Middle Jurassic—Lower Cretaceous and Upper
Cretaceous. Their ranges and the interrelationships among
them were formed by multi-stage Alpine processes of uplift-
ing of the area and its subsequent erosion (Moryc 2006;
Krajewski et al. 2011). Those movements caused reductions
in the sedimentation profile of the Mesozoic cover (Gutowski
et al. 2007; Matyja 2009; Krajewski et al. 2011; Kosakowski
& Wróbel 2011; Kosakowski et al. 2011) and a limitation of
the range of occurrence of particular complexes, especially
the Permian-Triassic complex (Jawor & Baran 2004). That is
a result of erosion that started in the Late Triassic. The next
structural complex starts with the Middle Jurassic forma-
tions. The complex has the widest extent, and it is formed by
the Middle Jurassic, Upper Jurassic as well as the Lower
Cretaceous formations. The rocks above, belong to Upper
Cretaceous formations with erosional unconformity; the gap
is related to the regional deformation of the Austrian phase
in the Aptian and Albian time.
The sandy Cenomanian strata begin the Upper Cretaceous
section. The remaining part of the profile is composed of car-
bonate formations. In the Late Cretaceous—Early Paleogene,
as a result of the Laramian phase, the study area was uplifted
and underwent intensive erosion (Jawor & Baran 2004). The
erosion lasted throughout the Paleogene time and resulted in
Fig. 1. Extent of the lowermost Mesozoic strata in the study area with location of 1-D modelled wells. Rus. – Russia, Lith. – Lithuania,
MSFZ – Moravian-Silesian Fault Zone, HF – Hana Fault, KLFZ – Kraków-Lubliniec Fault Zone, HCF – Holy Cross Fault, RRF – Rava
Ruska Fault, TTZ – Teisseyre-Tornquist Zone, ŁR – Łysogóry Region, KR – Kielce Region.
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the removal of the Upper Cretaceous strata from a
significant part of the study area. The Laramian ero-
sion also affected the formations of the Upper
Jurassic—Lower Cretaceous complex. The results in-
cluded significant differences in thickness between
the western part, where the thickness of that com-
plex reaches about 300 m, and the eastern part,
where its thickness is even 1300 m (Gutowski et al.
2007; Matyja 2009). The thickness of the terrige-
nous complex of Miocene age varies and increases
from the margin of the Carpathian Foredeep, so
that, for example, it amounts to over 1000 m in the
region of Tarnów, whereas in the region of Rzeszów
it is over 2500 m (Jawor & Baran 2004). From the
south, the flysch formations of the Outer Carpathians
were overthrusted onto the autochthonous Miocene
strata. Their thickness also increases from the mar-
gin of overthrusting towards the south. In the study
area, the thickness of the flysch strata ranges from a
few hundred meters to over 3800 meters (the area of
Nosówka).
Modelling procedure
1-D modelling of selected wells was performed
using BasinMod™ software (BMRM 1-D 2006).
The modelling approach adopted in the software re-
quires input data which describe the present-day
geological situation as a result of past events. On
this basis, the geological history is simulated from
the oldest event to the most recent one (Buła &
Habryn 2008, 2011). Rock properties – density,
porosity, permeability and thermal conductivity are
modelled along with the thermal history. BasinMod
software provides an extended database of various
lithological types defined by physical properties
mentioned above (BMRM 1-D 2006; Kosakowski
et al. 2012a). The details on principles of the model-
ling technique are given in Welte et al. (1997).
Thermal evolution is simulated on the basis of
boundary assignments applied to certain time steps.
The assigned parameters are heat flow densities in
mW/m
2
and surface temperatures in °C. Heat flow
and surface temperatures assignment for the past
stages of basin history can only be estimated based
on the general tectonic setting and evolution of the
investigated region (Besse & Courtillot 1991; Van
der Voo 1993; Yalcin et al. 1997; Allen & Allen
2005). To determine the magnitude of burial and
erosion Rock-Eval T
max
temperature and reflectance
of vitrinite (R
o
) data were used (Table 1). For burial
history reconstruction was also used: thickness of
individual stratigraphic units, numerical ages defin-
ing time interval between the upper and lower limit
of each stratigraphic unit, and petrophysical para-
meters for the individual units (compaction coeffi-
cient, initial porosity, thermal conductivity, heat
capacity). Estimation of eroded thicknesses has to
Table 1:
Vitrinite
reflectance
and
maceral
composition
of
the
Mesozoic
o
rganic
matter
in
the
selected
wells
(Kraków-Rzeszów
area).
OM
–
organic
matter
(sum
of macerals);
R
O
–
vitrinite reflectance;
R
Oredep
– redeposited organic matter;
Meas.
– number
o
f
measurements;
n.m.
–
not
measured;
n.d.
–
no
data;
tr.
–
t
races.
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be accompanied by testing various paleoheat flow models.
The thermal maturity of organic matter was calculated by the
EASY %Ro method (Sweeney & Burnham 1990). Genera-
tion and expulsion of hydrocarbons were calculated by the
LLNL model (Ungerer et al. 1988; Forbes et al. 1991;
BMRM 1-D 2006).
Modelling of maturation and generation history –
results and discussion
The 1-D maturity modelling as well as thermal and burial
history reconstruction were conducted for 7 wells: Będzieni-
ca 2, Dębica 10K, Góra Ropczycka 1K, Goleszów 5, Nawsie 1,
Pławowice E1 and Pilzno 40 (Fig. 1). The analysed Middle
and Upper Jurassic strata together with Lower Cretaceous
strata (Berriasian and Valanginian), form one complex of
carbonate sediments separated from the under- and overlying
ones by discordances. This complex is represented by
Oxfordian marls and marly limestones overlain by a com-
plex of bedded and massive limestones, Kimmeridgian pelitic
marly limestones and marls and Tithonian massive carbon-
ates developed in coral-sponge-microbial facies (Krajewski
et al. 2011). In the study area the Lower Cretaceous deposi-
tional sequence can be divided into two main facies: Berriasian
peloidal-microbial-cyanobacterial facies and Valanginian
ooidal-bioclastic facies (Zdanowski et al. 2001; Gutowski et
al. 2007; Urbaniec et al. 2010).
The model of the recent thermal regime was calibrated with
data obtained from maps of temperatures at the given depth
horizons (Majorowicz & Plewa 1979; Majorowicz et al. 1984;
Karwasiecka & Bruszewska 1997; Kotarba et al. 2004). More-
over, the analysis also takes into account the temperature mea-
surements from adjacent areas, namely the Upper Silesian
Block and Lublin Trough. In both areas, the distributions of
the thermal field and their reconstruction indicate much lower
Fig. 2. Burial history curves of the (A) Goleszów 5, (B) Pławowice 1, (C) Dębica 10K, (D) Góra Ropczycka 1 and (E) Pilzno 40 wells and
(F) Będzienica 2 wells. J
2
– Middle Jurassic, J
3
– Late Jurassic, Cr
2
– Late Cretaceous, M – Miocene, Outer Carp. – Outer Car-
pathians, Q – Quaternary.
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heat flow values and relative stability of paleothermal condi-
tions in the Mesozoic stage of basin development (Belka
1993; Botor et al. 2002; Kotarba et al. 2004).
The calculated values of recent heat flow across the study
area ranged between ca. 50 mW/m
2
in the eastern part and
ca. 60 mW/m
2
in its western and central parts.
The maturity modelling was calibrated with thermal maturi-
ty measurements, Rock-Eval T
max
temperature (Kosakowski
et al. 2012b) and vitrinite reflectance R
o
(Table 1). A signifi-
cant incompleteness in the stratigraphic section in the study
area makes it impossible to create one unique thermal—ero-
sional model. It is worth stressing, that in each of the analysed
models there is the possibility to use the alternative model
with an other scheme of the thermal and erosion evolution,
which in consequence gives a similar recent thermal maturi-
ty of organic matter. In view of the above-mentioned points,
Fig. 3. Maturity evolution curves for the Jurassic source rocks in profiles of analysed wells.
Fig. 4. The presumably extent of the “oil window” in the Jurassic and Cretaceous strata in
the Kraków-Rzeszów area.
the selection of a model for analysing
hydrocarbon generation and expul-
sion processes is, to a large extent,
subjective and gives an opportunity
for a different interpretation of the
course of petroleum processes in the
study area.
Considerations were based on the
model of thermal changes presented
by Narkiewicz et al. (2010), who
suggested constant heat flow during
the Permian, Mesozoic and Cenozoic
times.
The pre-Permian stage of basin de-
velopment, presented by Kosakowski
& Wróbel (2011), was ignored in the
reconstruction, as one not having a
significant impact on the develop-
ment of organic matter maturity in
the Jurassic strata.
The model of constant heat flow
over time equal to that of recent times
is sufficient to explain the available
thermal maturity measurements in the
Jurassic strata, because in the Meso-
zoic the thermal history of the study
area is relatively stable.
The key role in the evolution of or-
ganic matter maturity was played by
the deposition of thicker Upper Juras-
sic strata, and, above all, by the over-
thrust of flysch deposits of the Outer
Carpathians. The deposition of the Ju-
rassic strata placed the layers of source
rocks at the depth with the temperature
range of 60—80 °C, which represents
the beginning of the early mature
phase in the “oil window” (Figs. 2, 3).
Only in the wells located farthest north
of the Outer Carpathian boundary,
namely in the Pławowice E1 and
Goleszów 5 wells, the temperatures
were much lower and did not exceed
30—40 °C (Fig. 2A,B). The deposition of the Cretaceous strata
did not cause a significant increase in temperature, to a maxi-
mum of 50 °C. The post-Cretaceous uplift and erosion of the
study area stopped the increase in temperature, and consequent-
ly, the increase in organic matter maturity (Fig. 3). The deposi-
tion of the Miocene strata also did not cause big changes in the
Jurassic organic matter maturity. This is the result of both the
small thickness of Miocene rocks and low heat flow in the sedi-
mentary basin. Only the Outer Carpathian Overthrust placed the
layer of source rocks in the temperature range which determine
entering the initial phase of the “oil window” (0.5—0.7 %R
o
)
(Fig. 3). The maximal values of maturity reached by organic
matter in the Jurassic strata range from 0.6—0.65 %R
o
in the re-
gion of Bochnia-Tarnów-Dębica (Fig. 2C) to about 0.8 %R
o
in
the
south-west of Dębica, under the Carpathian Overthrust
(Fig. 2F). The thermal modelling has proven that the extent of
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maturity of the organic matter within
the “oil window” is not exactly the
same as the extent of the Carpathian
Overthrust; for example in the Dębica
area, the organic-matter maturity was
also influenced by the Miocene deposi-
tion (Fig. 4). Nevertheless, it can be
stated, in general, that attainment of ma-
turity in the phase of the “oil window”
is related to the overthrust of the Outer
Carpathians (Fig. 2C,D).
In the Mesozoic profile in the south-
eastern part of Poland only the Middle
Jurassic strata show rock complexes
that meet the quantitative criteria of
source rocks (Kosakowski et al. 2012b).
The geochemical analysis performed in
those strata revealed that the Triassic,
Upper Jurassic and Cretaceous strata
present generally very low TOC and hy-
drocarbon (S
1
+ S
2
) contents, and low
thermal maturity of organic matter addi-
tionally reduced their source rock po-
tential. The Middle Jurassic source
rocks show much higher TOC and hy-
drocarbon contents up to 17.0 wt. %
and 53.4 mg HC/g rock, respectively
(Kosakowski et al. 2012b). This poten-
tial is variable, but the maximum values
indicate the presence of good and very
good source rocks. Organic matter in
the Middle Jurassic strata is of mixed
type, dominated by gas-prone Type III
kerogen. The organic matter is imma-
ture, or mature in the early phase of the
“oil window”. The maturity of kerogen
increases towards to Outer Carpathians
(Kosakowski et al. 2012b).
This brief geochemical study of the
Mesozoic profile showed that only the
Middle Jurassic strata fulfil the criteria
for source rocks and the kinetic model-
ling were carried out only for this strata.
Modelling of hydrocarbon generation
from the Middle Jurassic source rocks
revealed that they only locally reached
the generation stage. In the predominant
part of the study area the transformation
degree of organic matter is low, below
10 % (Fig. 5). It was only in the eastern
part of the study area, where the source
rock formations are deeply submerged
under the Carpathian Overthrust and
reached the highest maturity, that the
transformation degree made it possible
to initiate the hydrocarbon generation
process.
In the Nawsie 1 well, the Middle
Jurassic source rocks reached the early
Fig. 5. Transformation ratio of kerogen in the Jurassic source rocks in the profiles of
analysed wells.
Fig. 6. A – Burial history curves for Jurassic source rocks with generation stages and
B – total amount of hydrocarbons generated from the Jurassic source rocks in Nawsie 1
well. For the abbreviations see Fig. 2.
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phase (10—25 % of generation potential) during the orogenic
phase of the Carpathian Overthrust, at a burial depth below
2300 m and at a temperature above 90 °C (Figs. 5, 6A). In that
well the source rocks also reached the main phase (25—65 %
of generation potential). This phase was reached at the end of
the Carpathian thrust belt, with the maximum of 5000 m and
the maximum temperature of 120 °C (Fig.6A).
In the remaining wells the initiation of the hydrocarbon
generation processes was not obtained, due to maturity being
below the threshold of 0.5 %R
o
.
The differences in the degree of transformation of kerogen
observed in the kinetic modelling also had an impact on the
generated hydrocarbon masses. Because the generation pro-
cess developed only in the Nawsie 1 well, the amount of the
obtained hydrocarbon mass was about 220 mg/g TOC
(Fig. 6B). In the resulting hydrocarbon mass the liquid phase
is dominant. In the remaining wells, the amount of the hydro-
carbon mass is minimal, usually below 10 mg HC/g TOC.
The expulsion phase is observed only in the Nawsie 1 well
(Fig. 6B).
Conclusions
In the Mesozoic profile of the south-eastern part of Poland
only the Middle Jurassic strata fulfill the quantitative criteria
for source rocks. The hydrocarbon potential of the Middle
Jurassic strata is variable, but the maximum values indicate
the presence of good and very good source rocks.
The burial and thermal history and generation modelling
with a determination of the amount of generated of hydrocar-
bons revealed that source rocks in the Middle Jurassic strata
of the basement of the Carpathian Foredeep were effective
only in a part of the study area. The analysis of the distribu-
tion of organic matter maturity and its evolution showed that
only in the eastern part of this area favourable conditions oc-
curred for mass generation of hydrocarbons. In this part of
the study area the source rocks reached the generation pro-
cess in the early and the main phase of the “oil window”.
The initial phase of generation was generally reached at the
stage of the Outer Carpathian overthrusting on the foreland.
Only in the Nawsie 1 well the source rock reached the initial
phase of the “oil window” during the deposition of the Upper
Cretaceous strata. The main phase of the “oil window” was
reached at the orogenic stage of the Carpathian Overthrust.
The maximum transformation degree was 60 %. The amount
of hydrocarbons generated from source rocks was propor-
tional to the transformation of the organic matter and it
reached 220 mg HC/g TOC.
The obtained modelling results clearly indicate that the
Middle Jurassic strata, with the heat flow constant over time
and equal to that found in recent times, can reach the transfor-
mation of organic matter necessary for the initiation of the
hydrocarbon generation process only at depths below 5000 m.
Acknowledgments: The research was undertaken as research
Project No. UKRAINE/193/2006 of the Ministry of Science
and Higher Education carried out at the AGH University of
Science and Technology in Kraków and Polish Geological
Institute – National Research Institute in Warsaw. The scien-
tific work was financed from the scientific fund in the years
2007—2010. The authors thank Izabella Grotek from Polish
Geological Institute – National Research Institute in Warsaw
for measurements of vitrinite reflectance and maceral compo-
sition. The authors want to express their sincere thanks to
Tadeusz Peryt (Polish Geological Institute – National
Research Institute), Paweł Karnkowski (University of War-
saw) and to the anonymous reviewer for their valuable com-
ments, which helped to prepare the final text.
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