GEOLOGICA CARPATHICA, 52, 5, BRATISLAVA, OCTOBER 2001
263 — 275
VARIATION OF DEFORMATION MECHANISMS WITHIN THE
PROGRESSIVE—RETROGRESSIVE MYLONITIZATION CYCLE OF
LIMESTONES: BRUNOVISTULIAN SEDIMENTARY COVER (THE
VARISCAN OROGENY OF THE SOUTHEASTERN BOHEMIAN MASSIF)
PETR ŠPAČEK
1*
, JIŘÍ KALVODA
1
, EVA FRANCŮ
2
and ROSTISLAV MELICHAR
1
1
Department of Geology and Paleontology, Masaryk University, Kotlářská 2, 61137 Brno, Czech Republic; *vajgl@sci.muni.cz
2
Czech Geological Survey, Leitnerova 22, 60200 Brno, Czech Republic
(Manuscript received December 7, 2000; accepted in revised form June 13, 2001)
Abstract: This study deals with the calcite mylonites of the Brunovistulian sedimentary cover developed in the frontal
thrust area of the Moravian nappe units. The inhomogeneous structure of sedimentary protoliths allowed the analysis of
the contrasting behaviour of calcite in matrix and porphyroclasts and the interpretation of microfabric evolution during
deformation under low temperature conditions. Several stages of microfabric evolution characterizing progressive as
well as retrogressive deformation are distinguished. Generally, the progressive phase of mylonitization is characterized
by grain growth in the matrix and the grain size reduction of the porphyroclasts leading to a stress-induced equilibration
of grain size. During the initial deformational stages the calcitic porphyroclasts deformed brittlely and the strain was
strongly localized into the ductile matrix. With continuing evolution the onset of the dynamic recrystallization of
porphyroclasts occurred, which obviously preceded a significant grain growth in the matrix. With rising temperature
during deformation, grain growth predominated after grain size homogenization was finished. The lack of effective
dynamic recovery along the stages of the progressive low temperature phase of deformation is discussed. Core-and-
mantle structures which are characteristic of the initial stages of progressive deformation carry microfabric features
which document the dominance of grain boundary bulging and/or nucleation recrystallization. Formation of subgrains
within the porphyroclasts is only a rarely observed feature which probably could not lead to significant grain size
reduction. The higher effectiveness of nucleation and recrystallization via migration of grain boundaries compared to
subgrain rotation mechanism could be a consequence of high fluid content. Large-scale thrusting within the Brunovistulian
basement is shown by the juxtaposition of calcitic and quartzitic mylonites with deformational microstructures reflecting
pronounced contrasts of deformational styles. Fully plastic vs. fully brittle behaviour of quartz represents the most
pronounced indicator of different deformational conditions between the lower unit of the Svratka Dome and the other
domains of the Brunovistulian basement. In the lower tectonic unit of the Svratka Dome the microtructures of calcite
mylonites indicate stresses which were about four times lower than in the other two parts of the Brunovistulicum. Despite
the deformational contrasts, the values of illite crystallinity measured do not show any spatial gradient which could be
linked with the distribution of the contrasting deformational microstructures. The paleothermometric data which are
available to date suggest maximum paleotemperatures of 250—300 °C for all three studied domains of the Brunovistulian
basement and it is suggested that the difference of Variscan peak temperatures between the three compared domains of
the basement was not higher than several dozens of °C. The observed deformational contrasts can thus be explained by
an abrupt change of deformation mechanisms in both calcite and quartz at temperatures around 300 °C.
Key words: Eastern Variscan front, Brunovistulicum, inhomogeneous limestones, mylonitization, dynamic recrystal-
lization, microstructures.
Introduction
Microfabric studies of strained homogeneous calcite aggre-
gates have been described relatively frequently, both in nature
(e.g. Dietrich & Song 1984; Heitzmann 1987; Burkhard 1990;
Covey-Crump & Rutter 1989; Busch & Van der Pluijm 1995)
and experiments (e.g. Schmid et al. 1977, 1980, 1987; Rutter
1974; Rutter et al. 1994; Walker et al. 1990). However, re-
search into the mylonitization of inhomogeneous carbonates,
which are the most abundant in nature, is rather sparse. There-
fore we attempted to give a detailed study of the development
of such inhomogeneous limestones in low-temperature (LT)
deformational stages.
In the southeastern part of the Bohemian Massif, the tecton-
ic contact of the allochthonous domain of Variscan orogen (the
Moldanubian and Moravian nappe units) and the per-autochth-
onous pre-Variscan basement (the Brunovistulicum) is ex-
posed (Matte et al. 1990). The Devonian and Lower Carbonif-
erous carbonate-clastic sedimentary cover of the Brunovistuli-
cum is strongly sheared in the thrust area under anchimeta-
morphic and very low-grade metamorphic conditions (Schul-
mann et al. 1991). Calcite mylonites from this highly de-
formed sedimentary sequence were studied along orogen-per-
pendicular profiles, which cross-cut the foot-wall of the
Moravian nappe units and proximal parts of their foreland.
As the microstructure of sedimentary protoliths was gener-
ally inhomogeneous, the mylonites served as a suitable object
for the comparison of the deformational behaviour of the ma-
trix vs. the porphyroclasts within the given spectra of LT de-
formational conditions. The analysis of deformational micro-
fabric allowed the interpretation of its evolution during the
progressive transformation of limestones into mylonites and
VARIATION OF DEFORMATION MECHANISMS WITHIN THE
PROGRESSIVE—RETROGRESSIVE MYLONITIZATION CYCLE OF
LIMESTONES: BRUNOVISTULIAN SEDIMENTARY COVER (THE
VARISCAN OROGENY OF THE SOUTHEASTERN BOHEMIAN MASSIF)
264 ŠPAČEK et al.
during retrogressive degradation under decreasing tempera-
tures. On the basis of the observed deformational microstruc-
tures it was possible to make a comparison between three do-
mains of the Brunovistulicum in terms of dominant deforma-
tional regimes in calcite aggregates.
Geological settings
The Variscan assembly of the allochthonous units and the
Brunovistulian basement within the eastern Bohemian Massif
are related to the Devonian-Late Carboniferous dextral oblique
collision of the Armorican terranes (Moldanubian and
Saxothuringian Terrane) with the Brunovistulian Terrane –
outer part of Laurussia (Matte et al. 1990; Kalvoda 1995,
2001). Three main units have been distinguished in the colli-
sional zone: Moldanubicum (Suess 1912) with high grade
Variscan metamorphism (Suess 1912, 1926; Cháb & Suk
1977), Moravian Zone (Suess 1912) with medium grade
Variscan metamorphism (Suess 1912, 1926; Štípská & Schul-
mann 1995) and Brunovistulicum (Dudek 1980), in which the
Variscan metamorphism is low-grade and occurs only in a
close contact with the overlying tectonic units (Schulmann et
al. 1991; Franců et al. 1999). According to some authors the
nappe units of the Moravian Zone were derived from the high-
est parts of the imbricated Brunovistulian basement (e.g. Frasl
1983; Fritz & Neubauer 1993; Štípská & Schulmann 1995), as
indicated mainly by similar radiometric ages of the Brunovis-
tulian granitoids and sheared orthogneiss bodies of the Mora-
vian nappes (van Bremen et al. 1982; Morauf & Jäger 1982).
The structure of the southern part of the collisional zone is
well exposed in two incomplete tectonic windows: the Thaya
Dome in the south and the Svratka Dome in the north (Fig. 1).
A similar lithotectonic zonation has developed in both of
them, as described, for example, by Schulmann et al. (1991,
1994) and Fritz & Neubauer (1993):
1 (bottom). Granitoids, metagranitoids and migmatites of the
Brunovistulian Cadomian basement with their metasedimentary
host rocks and Paleozoic sedimentary cover (Dudek 1980; Fin-
ger et al. 1989, 1995; Bosák 1980; Batík & Skoček 1981),
2. Moravian nappe units composed mostly of metasedi-
ments, pre-Variscan Bíteš orthogneiss and its metasedimentary
host rocks (e.g. Schulmann et al. 1991),
3. Mica-schist zone with metasediments, amphibolites and
orthogneiss bodies (Suess 1908),
4 (top). Moldanubian nappes with high-grade granulites,
paragneisses, migmatites and relics of eclogites (Matějovská
1975; Jenček & Dudek 1971; Vrána et al. 1995).
Fig. 1. Schematic map of the area studied and a conceptual profile through the main units of the collision zone.
DEFORMATION MECHANISMS WITHIN THE MYLONITIZATION OF LIMESTONES 265
Characteristic features of this sequence are inverted Bar-
rovian metamorphic zoning, metamorphic foliation parallel
with lithological boundaries and N to NE trending lineations
subparallel to the axes of tight folds (Schulmann et al. 1991).
In the upper units, E-W stretching lineations are common
(Fritz & Neubauer 1993).
In the foreland of the Moravian and Moldanubian nappe
units, the Brunovistulian basement is exposed in the Brno
batholith and has been verified through many boreholes be-
neath the Paleozoic cover on the eastern slopes of the Bohemi-
an Massif. In this eastern part of the collisional zone different
lithotectonic zonation is developed:
1 (bottom). Cadomian granitoids of the Brunovistulicum with
its metamorphosed host-rocks and Devonian-Lower Carbonif-
erous pre-flysh sedimentary cover (e.g. Dudek 1980; Leich-
mann 1996; Hanžl & Melichar 1997; Finger et al. 2000;
Dvořák 1995),
2. several km thick flysh sequence of Viséan age (Dvořák
1973; Rajlich 1990; Čížek & Tomek 1991).
The Viséan flysh sequence is strongly folded (e.g. Rajlich
1990) and Čížek & Tomek (1991) proved the existence of
large-scale east-vergent thrusts imbricating both the flysh se-
quence and the Brunovistulian basement with its tectonized
pre-flysh sedimentary cover. In this part of the orogen, the duc-
tile deformation of the rocks is non-penetrative and thick zones
of mylonitization occur only in close proximity to the Moravi-
an nappes. Stretching lineation and associated kinematic indi-
cators show top-to-the-NNE shearing (e.g. Bábek & Janoška
1997). In general, the degree of Variscan deformation and
metamorphism is very low and further decreases to the east
where Paleozoic sequences rest autochthonously on the Bruno-
vistulian basement.
Within the Brunovistulian basement, two parts with different
development during the Variscan orogenesis can thus be distin-
guished. The first is in the westernmost part with the Moravian
nappes in the hanging wall and the second in the eastern part is
covered by Viséan flysch nappes. The boundary of these two
sections is covered by Westphalian-Autunian sediments of the
Boskovice Graben. The exact meaning of the tectonic contact
of units beneath the sedimentary infill of the graben is still not
well understood.
For the tectonic evolution of the collisional zone the forward
thrust propagation model was suggested by Schulmann et al.
(1991), Fritz & Neubauer (1993) and Fritz et al. (1996). The
thrusting began under HT conditions and continued during
gradual cooling to LT conditions. The deformation regimes
were changing continuously from top-to-the-N shear through
top-to-the-E shear to E-W coaxial extension. The simultaneous
activity of non-coaxial shearing in the lower units and the co-
axial extension in the upper units has been assumed. This mod-
el explains the complex structural evolution and systematic de-
crease of isotopic ages of metamorphism from the uppermost
tectonic to the lowest tectonic levels.
Analytical methods
The transformations of the primary structures of inhomoge-
neous carbonate sediments into a deformation fabric of carbon-
ate mylonites were analysed. Dozens of samples were collect-
ed in both parts of the basement – from the foot-wall of
Moravian nappe unit in the western part and from the foreland
of the Moravian nappes in the eastern part of the basement
(Figs. 1 and 6). The key steps in the analytical procedure,
which should have provided data for the interpretation of de-
formation mechanisms and conditions, were:
1) the description and quantification of the optical deforma-
tion microstructures and lattice preferred orientations (LPOs);
2) the correlation of the microfabric with the temperatures
of deformation.
Microstructures
Thin and ultra-thin (< 10 µm) sections were prepared from
oriented samples cut parallel to XZ and ZY planes of finite
strain and were examined under optical and SEM micro-
scopes. Grain-shape analyses of the coarse-grained domains
were carried out using a polarizing microscope—digital cam-
era—computer arrangement. Images of the thin sections were
captured in two or three different polarizer/analyzer positions
in order to identify the maximum number of grain-boundaries
(Burkhard 1990). The two or three images obtained were pro-
jected on a horizontally oriented screen in a slideshow mode
and the grain boundary networks were then produced by man-
ually outlining the grains onto transparent foil. For the SEM
morphological analyses of the fine-grained aggregates, pol-
ished XZ and XY slabs of the selected samples were etched in
a 1% hydrochloric acid solution for 10 seconds and coated
with gold-film. Secondary electron photomicrographs were
obtained from 30—50° tilted samples after tilt-correction.
Quantitative processing of the grain boundary networks was
carried out using ImageTool 2.0 software. In this paper, only
the grain size parameter is used for the characterization of mi-
crostructures. The grain size (D) is defined as the diameter of
a circle with the same area as the grain being measured, that is
D = sqrt(4
×
grain area/
π
).
Such a definition of grain size gives the most realistic val-
ues which are independent of grain shape. For stress calcula-
tions we used the Rutter paleopizometer (Rutter 1995) calcu-
lated for the grain boundary migration (GBM) recrystal-
lization mechanism:
log
σ
= 2.22 + 0.37 log d — 0.30 (log d)
2
,
where
σ
is the differential stress and d is the grain size, and
the median values of grain size were used as suggested by
Ranalli (1984).
The content of dolomite and other secondary phases was
examined with an electron microprobe in selected samples in
order to assess their potential influence on the deformational
processes.
The stretch (S = original length/finite length of the deformed
object) was measured at pressure fringes, deformed peloids
and ooids, boudinaged clasts and other strain-markers in order
to demonstrate the strain magnitude of the distinguished mi-
crostructural types.
Lattice Preferred Orientations (LPO)
If the evolution of the mylonites was to be reconstructed, it
was necessary to determine the mechanisms operative during
the deformation. Therefore the LPO were measured. Their in-
266 ŠPAČEK et al.
tensity is related to the magnitude of the intracrystalline defor-
mational mechanisms and their ratio to the other mechanisms
of deformation (e.g. Casey & McGrew 1999). X-ray diffrac-
tion texture analysis was used for the comparison of the fabric
geometries and intensities of the distinguished microstructural
types. The measurements were carried out in the laboratory of
of Military Technical Institute of Protection in Brno, using a
Siemens D-500 texture goniometer. Textures were measured
using reflection geometry on thin slabs of the rock which had
been cut parallel to the macroscopic foliation (XY plane). Fil-
tered CuK
α
1+2
rays were used and maximum tilt was 80°. The
data were further tilt-corrected, using a tilt scan on a powder
sample and processed with popLA software (Kallend et al.
1991).
Preliminary results have shown that the LPO patterns of all
samples are very similar and that it was not necessary to calcu-
late orientation distribution functions. The LPO intensities of
the samples measured were compared in the incomplete
(
Φ
= 0—80°) pole figures of (018) planes (e-poles).
Additionally, crystallographic orientations of the coarse
grains were measured in several thin sections using optical po-
larizing microscope with a U-stage. This “semi-domainal”
LPO analysis allowed the LPO of the porphyroclasts and that
of the whole samples to be measured separately.
Paleothermometry
The illite crystallinity of clay fractions from shales associat-
ed with the mylonitized limestones was measured in order to
estimate the maximum reached paleotemperatures. Clay-size
material was separated from 8 rock samples after removing the
cements such as carbonates, organic matter and iron oxides
(Jackson 1975). Clay fraction < 2 µm was collected by centrif-
ugation for determination of illite crystallinity. Oriented slides
were analysed both air-dry and after vapour glycolation using
X-ray diffractometer Philips PW 1830 (generator) and PW
3020 (goniometer) with 0.02° step from 2 to 50 °2Q. Illite
crystallinity index (IC) was measured as peak width in
∆
2
Θ
at
half maximum (PWHM) of the (001) basal reflection of illite
(Kübler 1967) using background stripping and peak-fitting.
The results were calibrated to international standards (Warr &
Rice 1994).
Microstructures and their interpretations
The results of microfabric analyses allow several basic
groups of (proto-)mylonites with similar features to be distin-
guished. In the following discussion, these groups of micro-
structures will be identified with the letters A—E. The inter-
preted mechanisms of deformation are shown in a schematic
diagram in Fig. 3.
Microstructures A.
Weakly deformed protoliths
Rocks of this type retain their original inhomogeneous
structure and the sedimentary attributes of their protoliths. The
most typical composition includes a micritic matrix (d ~ 4 µm)
and a wide-ranging assemblage of various parts of fossil or-
ganisms, which together with boudinaged veins and other con-
stituents composed of sparite, will be referred to as “porphyro-
clasts”.
Strain markers, for example, the calcite-filled pressure fringes
around quartz clasts and deformed peloids, indicate that matrix
suffered substantial strains with minimum stretch values up to
S = 4.5. In spite of this high degree of strain, the micrite in the
matrix does not exhibit substantial microstructural changes.
The coarse-grained porphyroclasts are not substantially in-
ternally strained and figure as rigid bodies passively flowing
in a ductile environment. Locally, book-shelf fracturing, mi-
croboudinage, twinning and only slight undulose extinction
within the coarse grains can be observed in the samples with
higher finite strains or with the load-bearing framework of
coarse grains. The distribution of the c-axes measured in por-
phyroclasts is random to strong with a single maximum near
the pole to the foliation, depending on the strain magnitude
(not shown in the figure, in strongly deformed types the c-axes
distribution is very similar to that in Fig. 2d). Bulk (whole
sample) X-ray LPO is much weaker, increasing with the high-
er volume of the clasts (Fig. 2a).
Fabric development of this microstructure took place in a
semi-ductile regime. Strain partitioning due to grain size inho-
mogeneity, with preferential localization into fine-grained ma-
trix, is characteristic. For the matrix, the interpreted dominant
mechanism of the deformation is grain boundary sliding
(GBS) with accommodation by diffusion transfer at grain
boundaries. The main arguments for GBS are negligible mi-
crostructural changes in spite of high strains and the weak
LPO. The high water content in the limestones during defor-
mation is indicated by frequent pressure fringes and stylolites
in the micrite. It is very likely that the fluids have played an
important role in the diffusive matter-interchange between the
grains and could thus have caused a substantial weakening of
the matrix. During the deformation, the strength of coarse
grained porphyroclasts was much higher than that of the fine-
grained matrix (compare Fig. 7a). Local high stress conditions
resulted in brittle fracturing, twinning and incipient intracrys-
talline slip within the porphyroclasts.
Microstructures B.
Protomylonites
A mantled porphyroclasts/matrix structure is characteristic
for this group (Fig. 7b). Core-and-mantle structure grains are
free of clay minerals and in most cases can be easily distin-
guished from the matrix which appears darker under transmit-
ted light. The bulging of the grain boundaries and the forma-
tion of oval-shape recrystallized grains (Fig. 7c) takes place
preferentially at twin lamellae and boundaries of clasts.
This type of microstructure is interpreted as a result of grain
boundary bulging (GBB) or nucleation recrystallization
(Drury & Urai 1990; Mercier et al. 1977). High aspect ratios
of the porphyroclasts were generated mainly by the superposi-
tion of GBM on the twin lamellae (Fig. 7b). Within the matrix,
non-distinctive grain growth up to d < 10 µm also indicates the
incipient activity of grain boundary migration. The formation
of subgrains and rotation recrystallization are less pronounced
and do not lead to significant reduction in grain size. Despite
the occurrence of mantled porphyroclasts, which one is tempt-
ed to interpret as the product of subgrain rotation, the lack of
recovery in the grains suggests the dominance of the GBB
DEFORMATION MECHANISMS WITHIN THE MYLONITIZATION OF LIMESTONES 267
and/or nucleation mechanisms of recrystallization. The recrys-
tallized grains produced by grain size reduction of the porphy-
roclasts are usually larger in size than those resulting from the
grain growth of the matrix micrite (Table 1). This discrepancy
can be explained by the low rate of GBM in the matrix grains
as a result of their low level of internal strain and/or the inhibi-
tory effect of the secondary phase (Olgaard & Evans 1988).
The LPO of these types of protomylonites have features simi-
lar to that of the microstructures A: a strong single maximum
of the c-axes close to the pole of foliation in the porphyro-
clasts, which is weakened in the LPO of the whole sample
(Fig. 2b,c,d). The activity of GBS is likely to have persisted in
both the matrix and the domains of recrystallized grains as in-
dicated by the lack of microstructural change in spite of strong
deformation of the fine-grained domains. Boudinaged bio-
clasts indicate minimum stretch values of S = 6.1.
Microstructures C.
Mylonites
These types of rocks are composed of a relatively coarse-
grained matrix (d = 20—50 µm) with relict porphyroclasts. Pres-
sure fringes indicate minimum stretch values of S = 6.0. Grain
aspect ratios vary between 1.5 and 4. All the grains of the ma-
trix and the porphyroclasts are optically strain free, grain
boundaries are almost straight, slightly curved or bulbous.
Twin lamellae are rare, straight and were probably produced
during cooling due to high thermoelastic anisotropy of calcite
(Rosenholtz & Smith 1949). The LPO is similar both for ma-
trix and porphyroclasts, showing single maximum of e-poles
(and c-axes respectively) close to the pole of foliation (Fig.
2e). Because the grains lack undulose extinction and a sub-
grain microstructure and the grain boundaries are frequently
bulbous, we attribute the finite microstructure to GBM-domi-
nant recrystallization. Nevertheless, twinning and/or disloca-
tion glide are also likely to have played a substantial role dur-
ing earlier phases of the deformation as indicated by high
aspect ratios and straight boundaries of the grains and the en-
hanced intensity of LPO.
Locally, sharply terminated prolate lens-shaped domains are
developed in these types of mylonites, representing strained
stems of Amphipora sp. These domains are composed of rela-
Fig. 2. Sample pole figures of e-planes and c-axes of the main microstructural types. All data are projected to the plane of foliation in
equal-area projection, lower hemisphere. a—c, e, f – X-ray diffraction data in incomplete pole figures; intensities are expressed as multi-
ples of a random distribution (m.r.d.). d – c-axes distribution of porphyroclasts in microstructure B. Contours at 0, 2, 4, 6, 8, 10, 12, 14,
16 and 18 %. Notice the strong LPO of porphyroclasts vs. weak LPO of whole sample in the microstructural types B and the increasing
intensity of the preferred orientation from Type B to Type D with relatively constant distribution geometry. The patchy pattern of the dis-
tribution is due to the high content of large grains in the samples.
Fig. 3. The interpreted dominant deformational mechanisms oper-
ative in the distinguished stages of mylonitized limestones. GBS
– grain boundary sliding, GBB – grain boundary bulging, DG
– dislocation glide, GBM – grain boundary migration, SGR –
subgrain rotation recrystallization, nucl. – nucleation, BPT –
brittle-plastic transition.
268 ŠPAČEK et al.
tively coarse grained calcite aggregates of equant, strain free
grains with slightly curved boundaries.
Microstructures D.
Coarse grained marbles
In the most mature mylonites mesoscopic indicators (sheath
folds, boudinaged clusters of dolomite) suggest stretch values
of S > 10. In these types characteristic homogeneous domains
are developed with a uniform grain size which varies with the
volume of the dispersed phyllosilicates and dolomite (Table
1). Porphyroclasts composed of calcite are absent. In the do-
mains with a small amount of secondary phases, the grain size
usually reaches 100—120 µm. All grains are strain free, having
slightly curved to lobate boundaries. Grain aspect ratios are
usually > 2.5 and occasionally domains with equant coarse
grains with grain boundaries meeting in 100—140° triple junc-
tions can be observed (Fig. 7d). The c-axes distribution pattern
shows a strong single maximum close to the pole of foliation
(Fig. 2f). Rare twin lamellae are straight, and were probably
produced during cooling. The microstructural features of these
types suggest the dominance of GBM recrystallization mecha-
nism. However, strong LPO indicates substantial activity of
intracrystalline deformation during the evolution of these
types, whose microstructures could have been overprinted in
the latest phases of the deformation.
Microstructures E.
Retrogressively deformed marbles
In some areas, grain size reduction of the coarse grains oc-
curs within D types and narrow shear zones are developed af-
fecting coarse-grained aggregates of microstructure D (Table
1). The old grains are polygonized into subgrains and newly
formed grains usually have a crystallographic orientation very
close to that of their host grains (Fig. 7e). As the grain bound-
aries of the recrystallized grains are interpenetrating and bul-
bous, we suggest that the grain size reduction is an effect of
the combination of both subgrain rotation and GBM mecha-
nisms. These structures are attributed to the onset of retrogres-
sive deformation during incipient cooling. Further low temper-
ature deformation of some domains generated strong twinning
and undulose extinction of the coarse grains.
Paleothermometry
Illite crystallinity was measured in clay fractions of eight
samples from both the Svratka and Thaya Domes and western
margin of the Brno batholith. Two samples were excluded
from further processing because of their high content of ex-
pandable smectite and chlorite.
The values of illite crystallinity index (IC) range from 0.20
to 0.35°
∆
2
Θ
(Table 2) and indicate higher part of very low-
grade metamorphic (VLGM) conditions with probable maxi-
mum paleotemperatures of 250—320 °C (calibration after Frey
& Robinson 2000). The thermal alteration is more advanced
than in most Paleozoic rocks of the Drahany Upland which
show mainly lower VLGM conditions (Franců et al. 1999).
The results of IC thermometry are consistent with the data of
Bosák (1984) who analysed the degree of kerogen graphitiza-
tion in dark carbonate rocks of the lower units of the Svratka
Dome and of the western margin of the Brno batholith. He
concluded that in most samples from the Svratka Dome the
maximum temperature did not exceed 300 °C and that the
grade of thermal alteration of organic matter was considerably
lower in the carbonates of the Brno batholith’s western mar-
gin. Similar conclusions were made recently by Ulrich (2000)
who analysed the carbon and oxygen isotopic composition of
six carbonate samples from two localities in the lowermost
unit of the Svratka Dome. Using the graphite-calcite thermom-
eter and calibration of Covey-Crump & Rutter (1989) he stated
that the maximum temperatures in the graphite-rich marbles
did not exceed 300 °C for a longer period of time. In the lime-
stones of the Brno batholith’s western margin paleotempera-
tures of 250—300 °C are indicated by the degree of conodont
Table 1: Grain size values and calculated paleostresses of selected typical samples of the calcite mylonites studied. In some domains,
stresses were not calculated for the reasons expressed by abbreviations: sp – high content of secondary phase (possible inhibition of
grain growth), nu – not well understood mechanisms of origin (inhomogeneous tectonofacies with ambivalent characteristics), ss –
non-recrystallized primary sedimentary structures, crm – combination of recrystallization mechanisms.
tectonic domain microstructure sample no., locality
microstructural domain (and responsive deformation phase)
d (µm, median)
σ
diff.
(MPa)
eastern
B
s88b, Čebín
matrix
4.0
ss
eastern
B
s88b, Čebín
recrystallized grain mantles (peak metamorphosis)
6.2
211
eastern
B
s90-1, Čebín
matrix
5.0
ss
eastern
B
s90-1, Čebín
recrystallized grain mantles (peak metamorphosis)
8.2
203
eastern
B
s51a, Lažany
matrix
5.41
ss
eastern
B
s51a, Lažany
recrystallized grain mantles (peak metamorphosis)
6.7
209
eastern
B
s188, Šebetov
recrystallized grain mantles (peak metamorphosis)
8.0
204
western
B
s45-1, Kadov
matrix
4.3
ss
western
B
s45-1, Kadov
recrystallized grain mantles (peak metamorphosis)
7.2
207
western
C
s170, Květnice
fine grained domains
12.3
nu
western
C
s170, Květnice
coarse grained domains
26.9
nu
western
C
s 239, Vohančice
fine grained domains
19.6
nu
western
C
s 239, Vohančice
coarse grained domains
27.3
nu
western
D
s166-1, Dranč
coarse grained domains (peak metamorphosis)
100.5
57
western
D
s171, Lažánky
fine grained domains
30.6
sp
western
D
s171, Lažánky
coarse grained domains (peak metamorphosis)
115.6
51
western
D
s158, Lažánky
coarse grained domains (peak metamorphosis)
89.4
63
western
D
s151, Dřínová
coarse grained domains (peak metamorphosis)
102.4
56
western
D
s157, Vohančice
coarse grained domains (peak metamorphosis)
111.5
52
western
E
s157, Vohančice
fine grained domains (incipient retrogression)
38.9
crm
western
E
s157, Vohančice
fine grained domains (advanced retrogression)
24.4
crm
DEFORMATION MECHANISMS WITHIN THE MYLONITIZATION OF LIMESTONES 269
Table 2: Illite crystallinity values of clay fractions from shales as-
sociated with the mylonitized limestones. BB – Brno batholith’s
western margin, TD – lower tectonic unit of the Thaya Dome, SD
– lower tectonic unit of the Svratka Dome. (*) – associated tec-
tonofacies are marked with capital letters in parentheses.
alteration. The black colour of the conodonts without the tones
of brown corresponds to conodont colour alteration index
(CAI) 5—5.5 (see Frey & Robinson 2000 for calibration).
Indirectly, and with limited reliability, the available paleo-
thermometric data which are summarized in Table 3 can be
supported by the features of deformation microstructures ob-
served in quartz. In metamorphosed basement crystalline
rocks and Devonian conglomerates and sandstones of the low-
er tectonic unit of the Svratka Dome, quartz aggregates carry
clusters of recrystallized quartz grains with a similar c-axis
orientation and intensely sutured grain boundaries. Well-de-
veloped low-angle boundaries and subgrains inside relic old
grains are commonly found (Fig. 7g). This fabric is indicative
of deformation by dislocation creep with recovery, subgrain
rotation recrystallization and grain boundary migration being
operative. The features of the microstructure thus correspond
to the fully plastic deformation regime 3 of Hirth & Tullis
(1992). After Stöckhert et al. (1999), the steady-state medium
stress dislocation creep of quartz in the fully plastic regime
can only be effective at temperatures above the closure tem-
perature for K-Ar and Rb-Sr systems of biotite, that is above
ca. 310±30 °C. In contrast, in the eastern tectonic domain,
quartz is brittlely deformed, lacking any traces of intracrystal-
line slip (Fig. 7h). We consider similar pressure of fluids dur-
ing the deformation of the quartz aggregates in both units. It
seems to be a reasonable assumption that in the eastern part of
the Brunovistulian basement (external part of the orogen) the
brittle quartz was not deformed at higher strain rates than the
plastic quartz in the lower tectonic units of the Svratka Dome
(more internal part of the orogen). Assuming this, the observed
deformational microstructures of quartz indicate that in the
eastern part of the Brunovistulian basement (Brno batholith’s
western margin), the deformation was taking place under tem-
peratures which were probably lower than 310±30 °C.
The lack of significant IC differences between the compared
domains of the Brunovistulian basement (Table 3) suggests
that the metamorphic transformation of smectite into illite
reached similar stages in the studied rocks of the Brno
batholith’s western margin, the Thaya Dome and the Svratka
Dome and that the paleotemperature differences are below the
detection limit of the IC paleothermometer.
Considering potential errors of the paleothermometers and
the variation of the IC values measured, it can be stated that
the maximum paleotemperatures under which the studied
rocks were deformed probably lie between 250 and 300 °C
(Table 3). As was discussed above, the deformational features
of both quartz and calcite indicate that in the Brno batholith
and the lower unit of the Thaya Dome the maximum pale-
otemperatures were somewhat lower than in the lower unit of
the Svratka Dome. However, the paleothermometric data con-
strain the maximum difference of Variscan peak temperatures
between the three compared domains of the basement to sever-
al dozens of °C only (see Table 3).
The development of mylonitic stages
The sequence of microstructures A—E which has been dis-
tinguished above can be seen as a succession of frozen-in stag-
es within the process of the deformational and metamorphic
transformation of sediments. Several facts justify such an
opinion: the analogous lithostratigraphic position of calcite
mylonites, their overlapping biostratigraphic ranges and the
mutual transitions of microstructural stages. A schematic dia-
gram of the model is presented in Fig. 4. It is necessary to
stress the fact that unquestionable primary sedimentary mark-
ers – fossil organisms – are common within the microstruc-
tures A, B and C. Microprobe analyses revealed a calcitic
composition of the fossils. This is the main argument for inter-
preting the A—D sequence as a product of progressive my-
lonitization under increasing metamorphic conditions. During
the retrogressive deformation phases, the fine-grained matrix
of Type C was probably reworked again, but a significant
change in the microstructure did not occur. The Type C micro-
structures never acquired the features of D types during its
Table 3: Table of paleothermometric data of the studied area which are collected from the available literature.
tectonic domain* lithology
locality
IC (
∆°2Θ)
BB (A)
clayey limestone
Újezd u B. (s168)
0.30
BB (A)
shale
Újezd u B. (s168b)
0.28
BB (B)
clayey limestone
Šebetov (s111)
0.25
BB (A)
shale
Chudčice (s161)
0.20
TD (B)
shale
Skalice (s221)
0.35
SD (D)
shale
Lažánky (s237)
0.24
Brno batholith’s western margin
Lower tect. unit of the Thaya Dome
Lower tect. unit of the Svratka Dome
graphite/calcite thermometer (Ulrich 2001 with calibration after Covey-Crump & Rutter 1989)
–
–
max. 300 °C
CAI (Špaček 2001, calibration after Frey & Robinson 1999)
>250 °C
–
–
graphitization of kerogen (Bosák 1984)
<300 °C
<300 °C
max. 300 °C
illite crystallinity (this work, calibration after Frey & Robinson 1999)
250–320 °C
250–320 °C
250–320 °C
dynamic recrystallization of calcite (this work, after Burkhard 1990)
min. 250 °C
min. 250 °C
>250 °C
plastic deformation of quartz (this work, after Stöckhert et al. 1999)
–
–
>310±30 °C
270 ŠPAČEK et al.
evolution. It was never fully homogenized and primary sedi-
mentary structures were not completely destroyed. Thus, only
the phase during which the microstructures E were produced is
interpreted as retrogressive. Generally, the progressive phase
of mylonitization is characterized by the grain growth of the
matrix and a grain size reduction of the clasts leading to a
stress-determined equilibrium of the grain size. With rising
temperature during deformation, the homogenization of grain
size was finished and grain growth predominated. In retrogres-
sive phase, grain size reduction occurred due to a decreasing
temperature and increasing stress.
Mechanisms of recrystallization
One of the most surprising features one can observe in the
mylonitized sequence of carbonates studied is the dominance
of GBM and the lack of effective dynamic recovery within the
microstructures of the progressive low temperature phase of
deformation.
Recovery represents the process of ordering the lattice de-
fects, originated during intracrystalline slip, into subgrain
boundaries which leads to a decrease in the internal strain en-
ergy of the crystal. When dislocations are continuously added
to subgrain boundaries, the misorientation of the subgrains in-
creases and new grains are formed. This process of new grains
formation is referred to as subgrain rotation recrystallization
(SGR) and produces diagnostic core-and-mantle structures
with (sub-)grains increasingly misoriented towards the exter-
nal parts of mantle (Guillopé & Poirier 1979; Lloyd & Free-
man 1994). If the temperature is high enough to enable order-
ing of the lattice defects, continuous recovery-accommodated
dislocation creep can operate. However, when the temperature
is too low, recovery cannot keep pace with the tangling of the
dislocations during intracrystalline slip, newly formed disloca-
tions cannot move and strain hardening of the lattice occurs
(e.g. White 1977).
In our study, small (d ~ 8 µm) recrystallized grains of the
mantled porphyroclasts in high stress mylonites B do not show
any optical filiation to the host grains and their shape indicates
the activity of GBB and/or nucleation (Fig. 7b,c). Although ul-
tra-thin sections were used for the observation of microstruc-
tures, the formation of small-sized subgrains within the coarse
grains was found only sporadically.
We therefore explain the recrystallization of the clasts in mi-
crostructures B as the product of a GBB-dominant process.
Our observations lead us to the conclusion that during the pro-
gressive, low temperature deformation of the limestones stud-
ied, SGR was not capable of reducing the coarse grains into a
steady-state size. Recovery and SGR produced only relatively
large (sub-)grains which must have been further reduced by
more effective GBB.
Fig. 4. Schematic diagram of microfabric development in mylonitized sequence of limestones. Notice the different peak grades reached
in the lower tectonic unit of the Svratka Dome and the other two domains of the Brunovistulian basement. Objects in diagrams: black –
quartz, gray – micrite and microsparite, white – coarse-grained calcite. BB – Brno batholith’s western margin, TD – lower tectonic
unit of the Thaya Dome, SD – lower tectonic unit of the Svratka Dome.
DEFORMATION MECHANISMS WITHIN THE MYLONITIZATION OF LIMESTONES 271
Fig. 5. The suggested model of recrystallization mechanisms in a
complete deformation path of mylonitized limestones. Individual
microstructures are marked with capital letters A—E. See text for
explanations.
A suggested model of recrystallization development is
shown in the Fig. 5. According to Lloyd & Freeman (1994),
the velocity of grain boundary migration processes is deter-
mined by the relative crystallographic characteristics of adja-
cent grains, the driving forces, temperature and the structure of
the boundary. Driving forces include mainly lattice defects,
elastic energy and grain-boundary energy, and always lead to a
decrease in internal strain energy. In our case, as the SGR did
not lead to sufficient grain size reduction, each increment of
continuing deformation raised the internal strain of the large
grains and could accelerate the grain boundary bulging. Hip-
pertt & Egydio-Silva (1996) presented arguments for the activ-
ity of solution-reprecipitation process during the deformation
of quartz which can be concurrent with solid state recrystalli-
zation. Thus the high content of water in the system, which is
indicated by frequent markers of solution transfer, probably
also significantly increased the GBB or nucleation rate (com-
pare also with Tullis & Yund 1982). The facilitating of grain
boundary migration resulting from a high water content would
explain the contradiction of our model to observations of some
other authors who suggest that SGR is more effective than
GBB under lower temperatures (Schmid et al. 1987). The re-
crystallization mechanisms of calcite in LT conditions could
be analogous to those of quartz, in which grain boundary mi-
gration-dominant structures have even been described for dry
samples (Hirth & Tullis 1992).
Deformational contrasts and the imbrication of the
Brunovistulicum
It has been demonstrated by many authors that inverse pro-
portionality between stress and recrystallized grain size exists
(e.g. Twiss 1977; Kohlstedt & Weathers 1980). Thus, under a
constant strain rate, the increase in recrystallized grain size is
due to a decrease in material strength. Analogously, grain size
distribution within a mylonitized sequence can be viewed as
the result of metamorphic grade (i.e. temperature) variation.
We therefore attempted to assess the differences between the
deformation grade of the two domains of the deformed Bruno-
vistulian basement. The most effective and reliable method of
relative paleostress estimation seems to be the comparative
measurement of grain size in the peak grade microstructures of
individual tectonic domains. Uniform recrystallized grain size
within broad domains justifies the presumption of steady state
creep (e.g. Twiss 1977; Michibayaschi 1993). Facies with
small-scale grain size variations were not taken into account in
the paleostress calculations. It was assumed that the coarsest
recrystallized grain size within the defined groups of micro-
structures represents the peak metamorphic conditions. In
many coarse grained domains of facies D, the lack of anneal-
Fig. 6. Simplified sketch of the studied area showing the distribu-
tion of distinguished microstructural types. Circles with numbers
indicate sampled localities which are referred to in the tables and
figures. 1 – Šebetov (s111), 2 – Újezd u Boskovic (s168, s168b),
3 – Lažany (s51a), 4 – Čebín (s88b, s90-1), 5 – Chudčice
(s2056, s161), 6 – Kadov (s45-1), 7 – Skalice (s221), 8 –
Lažánky (s171, s158, s237), 9 – Vohančice (s157, s239), 10 –
Květnice (s170), 11 – Dřínová (s151) and Dranč (s166-1).
272 ŠPAČEK et al.
Fig. 7. Photomicrographs of characteristic deformational microstruc-
tures in calcite mylonites and quartz. A – Strained grainstone with pe-
loids and syntaxially overgrown crinoids. The contrasting strengths of
peloids and coarse spar and localization of the strain into micrite are ap-
parent. Plane polarized light. B – Protomylonite (type B) with core-
and-mantle structures. Note the localization of recrystallization into
twin boundaries of the clast. Crossed polarizers. C – Detail of mantled
porphyroclasts and oval-shaped recrystallized grains nucleating in and
bulging into the clast. 45° crossed polarizers. D – Domain with sub-
equant grains in the tectonofacies D, representing the peak-grade micro-
structure of the western part of the basement. Curved and bulbous grain
boundaries of indicate GBM process. Crossed polarizers. E – Recov-
ery and SGR recrystallization in retrogressive tectonofacies E. F –
Brittle fracturing of quartz in limestones of the eastern part of the base-
ment. Crossed polarizers. G – Recrystallization of quartz by SGR and
GBM typical for the western part of the basement. Crossed polarizers.
DEFORMATION MECHANISMS WITHIN THE MYLONITIZATION OF LIMESTONES 273
ing is evidenced with the shape of the grain boundaries, internal
strain and polygonization of the grains. It can be stated that after
reaching peak temperatures and the localization of the retrogres-
sive deformation into narrow zones, no substantial grain growth
took place in the domains which are now coarse grained. The
stress calculations thus should not be affected by static recrystal-
lization. In Table 1, the calculated paleostresses are given for
several typical samples, using the Rutter paleopiezometer (Rut-
ter 1995) for the GBM recrystallization mechanism.
If we compare the stress values of the facies B and D, which
represent the peak metamorphic conditions in the eastern and
western parts of the Brunovistulian basement respectively, we
can see a significant difference. Stresses four times lower in the
lower tectonic unit of the Svratka Dome than in the other two
parts of the Brunovistulicum are in accordance with the ob-
served deformation regimes of quartz. As the three compared
parts of the Brunovistulian basement are eroded to a similar
lithostratigraphic level, the tectonic juxtaposition of the con-
trasting facies must have occurred during late tectonic phases.
The main contrasts however, are not seen between the two parts
of the Brunovistulicum with different tectonostratigraphic zona-
tion, which were defined above, but they lie between the lower
tectonic unit of the Svratka Dome and the other two domains of
the Brunovistulicum – the Brno batholith’s western margin
and the lower tectonic unit of the Thaya Dome (Fig. 6).
Summary and concluding remarks
The analysis of the mylonites assembly developed within
the major thrust system of the Central European Variscan
orogeny revealed several characteristic features:
1) A lack of effective dynamic recovery within the progres-
sive low temperature phase of deformation. Microstructural
features of core-and-mantle structures developed in calcite
protomylonites provided evidence of GBB-dominance of the
recrystallization process. In this phase, the SGR mechanism
produced only relatively large grains, which must have been
further reduced by GBB and/or nucleation. Recovery was ef-
fective only during grain size reduction in the retrogressive
phase. This can be explained with a higher rate of GBB under
lower temperatures, which could have been increased as a re-
sult of a high fluid content.
2) The onset of grain size reduction of porphyroclasts prior
to distinct grain growth in matrix.
During the incipient mylonitization of inhomogeneous mi-
critic limestones, the porphyroclasts and matrix display con-
trasting rheological behaviour and strong strain localization
into a superplastic matrix occurs. At a certain point of mylo-
nite development, which is probably temperature-determined,
GBB is facilitated and the steady-state dynamic recrystalliza-
tion of clasts sets in. The recrystallized grain size is very close
to the grain size in the matrix. Assuming that an inverse pro-
portionality between grain size and stress is valid, the exist-
ence of approximate stress homogeneity must be considered in
naturally deformed calcite aggregates. A distinct to almost
complete dynamic recrystallization of the porphyroclasts and
minimum microstructural changes of the matrix indicates sig-
nificant strain rate differences between the porphyroclasts and
the matrix.
3) Variscan large-scale thrusting within the Brunovistulian
basement is indicated by the juxtaposition of facies with con-
trasting microstructures which reflect incompatible peak-grade
conditions. The main deformational contrasts can be observed
between the lower tectonic unit of the Svratka Dome and the
other two domains of the Brunovistulicum – the Brno
batholith’s western margin and the lower tectonic unit of the
Thaya Dome.
It seems very likely that the recrystallized grain size within
the mylonitized sequence of limestones studied is due to dif-
ferential stress variations. Assuming this, it is quite surprising
that temperature differences probably not exceeding 50 °C re-
sulted in such dramatic changes of differential stresses and re-
sponsive microstructures (compare microstructures A and B
with D). Actually, we are not the first to have observed indica-
tions of such contrasting behaviour of calcite aggregates under
natural LT deformation conditions. Burkhard (1990) examined
the change of the microfabric of micritic limestones strained
under a natural temperature gradient. He found out that up to
250 °C, grain size distributions were indistinguishable from
the sedimentary protolith. Above 280 °C, an increase in grain
size in micritic limestones occurred along with an increase in
the preferred orientation of the lattice and grain-shape. Behr-
mann (1983) described distinct variations in the microfabric of
calcite mylonites strained at about 300 °C. Microstructural
features of the tectonofacial succession, which were described
above, provide evidence of the dominance of GBB process or
nucleation during the progressive part of LT mylonitization.
Burkhard (1990) also suggested a grain boundary migration
mechanism for grain growth in epizonally strained micrites.
Grain boundary migration has a first order dependence on tem-
perature (e.g. Guillopé & Poirier 1979) and it can be expected
that the variation of finite microstructures within the lime-
stones strained under LT conditions is due to a significant
change of GBB effectiveness at temperatures around 300 °C.
Acknowledgments: We thank the creators of ImageTool 2.0
for its free provision at http://www.uthscsa.edu/dig/
itdesc.html. The constructive reviews of K. Schulmann, D.
Plašienka and an anonymous reviewer are highly acknowl-
edged. The research was supported by Grant Agency of Czech
Republic through Grant No. 205/98/0751 and by research plan
J07/98:143100004.
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